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| Open AccessLight-driven C–H activation mediated by 2D transition metal dichalcogenides
C–H activation in long-chain organic molecules remains largely unexplored. Here, the authors report light-driven C–H activation mediated by 2D TMDCs and the resultant synthesis of luminescent carbon dots.
- Jingang Li
- , Di Zhang
- & Yuebing Zheng
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Article
| Open AccessPhase-resolved measurement and control of ultrafast dynamics in terahertz electronic oscillators
Researchers using femtosecond lasers generate offset-free THz pulses to phase-lock the electronic oscillators. This enables the phase-resolved measurement of the emitted THz pulses with sub-cycle time resolution. Ultrafast dynamic response, such as anti-phase locking behavior, is also observed.
- Takashi Arikawa
- , Jaeyong Kim
- & Koichiro Tanaka
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Article
| Open AccessTamm-cavity terahertz detector
Here the authors report a terahertz detector with a Q value of 1017, embedded in a Tamm cavity and offers a 469 MHz bandwidth. It features an Nb5N6 microbolometer in an Si/air DBR and metal reflector, with tunable resonant frequency via substrate layer thickness.
- Xuecou Tu
- , Yichen Zhang
- & Peiheng Wu
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Article
| Open AccessFacet-selective growth of halide perovskite/2D semiconductor van der Waals heterostructures for improved optical gain and lasing
Halide perovskite/2D transition metal dichalcogenides (TMD) heterostructures hold promise for photonic/optoelectronic applications, but their bottom-up growth remains challenging. Here, the authors report a van der Waals heteroepitaxy strategy to synthesize various halide perovskite/TMD heterostructures with enhanced lasing performance.
- Liqiang Zhang
- , Yiliu Wang
- & Xidong Duan
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Article
| Open AccessPerfect linear optics using silicon photonics
The Authors demonstrate a fidelity-restorable universal integrated linear optical circuit that relies on a novel 4 × 4 silicon photonic crossbar architecture. Its experimental characterization yields a fidelity of 99.93 ± 0.06%, calculated over 10,000 matrices.
- Miltiadis Moralis-Pegios
- , George Giamougiannis
- & Nikos Pleros
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Article
| Open AccessObservation of discrete-light temporal refraction by moving potentials with broken Galilean invariance
Here, authors construct a moving potential barrier in a synthetic temporal lattice. They unveil the selection rules for choosing potential moving speed as well as the conditions to achieve transparent moving potentials and refraction.
- Chengzhi Qin
- , Han Ye
- & Peixiang Lu
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Article
| Open AccessAmplification of electromagnetic fields by a rotating body
The Authors measure the amplification of electromagnetic waves scattered by a rotating metallic cylinder, gaining mechanical rotational energy from the body, as predicted by Zel’dovich in 1971.
- M. C. Braidotti
- , A. Vinante
- & H. Ulbricht
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Article
| Open AccessSpatiotemporal optical vortices with controllable radial and azimuthal quantum numbers
The authors demonstrate the experimental generation and mode conversion of spatiotemporal Laguerre/Hermite-Gaussian wavepackets with controllable dual quantum numbers by imprinting two-dimensional complex modulation onto the spectrum of ultrashort laser pulses, opening new possibilities for spatiotemporally sculpturing of light.
- Xin Liu
- , Qian Cao
- & Qiwen Zhan
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Article
| Open AccessObservation of heat pumping effect by radiative shuttling
Authors demonstrate a net heat flux between two objects at averagely zero temperature gradient, exploring the nonlinear thermal emissivity based on phase change materials.
- Yuxuan Li
- , Yongdi Dang
- & Yungui Ma
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Article
| Open AccessChameleon-inspired tunable multi-layered infrared-modulating system via stretchable liquid metal microdroplets in elastomer film
Liquid metal-based infrared-modulating materials and systems have been developed to regulate the infrared reflection with multiple modes, which can be used for infrared camouflage, programmable infrared encryption, and infrared painting/writing.
- Yingyue Zhang
- , Hanrui Zhu
- & Tao Deng
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Article
| Open AccessOn-chip photodetection of angular momentums of vortex structured light
Structured vortex light with orbital angular momentum (OAM) holds promise for various optical applications, but its on-chip electrical detection remains challenging. Here, the authors report the realization of photothermoelectric OAM detectors based on 2D PdSe2 and spin-Hall surface plasmonic polariton couplers.
- Mingjin Dai
- , Chongwu Wang
- & Qi Jie Wang
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Article
| Open AccessPlasmons in the Kagome metal CsV3Sb5
Plasmons polaritons, or collective excitations of electrons and electromagnetic fields, have been rarely studied in layered correlated materials. Shiravi et al. report hyperbolic plasmon polaritons in thin flakes of the Kagome metal CsV3Sb5 and discuss correlation effects on their formation and tunability.
- H. Shiravi
- , A. Gupta
- & G. X. Ni
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Article
| Open AccessRoom temperature, cascadable, all-optical polariton universal gates
A cascadable all-optical NOT gate is a requirement for full-logic in optical computing. By introducing the concept of non-ground-state polariton amplification in organic semiconductor microcavities, the authors realized the operation of an all-optical cascadable universal gate.
- Denis A. Sannikov
- , Anton V. Baranikov
- & Pavlos G. Lagoudakis
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Article
| Open AccessOvertone photothermal microscopy for high-resolution and high-sensitivity vibrational imaging
The authors develop overtone photothermal microscopy that leverages a pump-probe detection of second overtone vibrations within the shortwave-infrared (SWIR) window. This technique complements existing large-scale SWIR imaging approaches, offering enhanced resolution and sensitivity for bioimaging applications.
- Le Wang
- , Haonan Lin
- & Ji-Xin Cheng
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Article
| Open AccessRaman micro-spectroscopy reveals the spatial distribution of fumarate in cells and tissues
Methods for the analysis of metabolites in cells often require sample disruption and lack spatio-temporal resolution. Here, the authors show that Raman spectroscopy can directly detect fumarate in living cells and animal tissues ex vivo.
- Marlous Kamp
- , Jakub Surmacki
- & Sarah E. Bohndiek
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Article
| Open AccessCavity-enhanced single artificial atoms in silicon
The authors demonstrate a cavity enhancement of single artificial atoms at telecommunication wavelengths in silicon by coupling them to highly optimized photonic crystal cavities, showing intensity enhancement and highly pure single-photon emission.
- Valeria Saggio
- , Carlos Errando-Herranz
- & Dirk Englund
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Article
| Open AccessObservation of Boyer-Wolf Gaussian modes
Lasers drive modern research and technology. The modes of laser resonators are crucial for understanding complex cavities, beam propagation, and structured light. Here, the authors experimentally observe a new family of fundamental laser modes with inherent parabolic symmetry: the Boyer-Wolf Gaussian modes.
- Konrad Tschernig
- , David Guacaneme
- & Miguel A. Bandres
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Article
| Open AccessBirefringence-induced phase delay enables Brillouin mechanical imaging in turbid media
Non-contact Brillouin microscopy holds potential to disrupt mechanobiology, yet this method faces challenges in presence of strong Rayleigh scattering. Here, the authors introduce a common-path birefringent filter exhibiting ultra-high extinction ratio to investigate turbid biological samples.
- Giuseppe Antonacci
- , Renzo Vanna
- & Giulio Cerullo
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Article
| Open AccessLight-evoked deformations in rod photoreceptors, pigment epithelium and subretinal space revealed by prolonged and multilayered optoretinography
Optoretinography-based detection of phototransduction and cell deformations in the retina has been mostly centered on photoreceptors. Here, the authors use prolonged and multilayered optoretinography to study light-evoked deformations in rod photoreceptors, retinal pigment epithelium, and subretinal space.
- Bingyao Tan
- , Huakun Li
- & Tong Ling
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Article
| Open AccessDirect bandgap quantum wells in hexagonal Silicon Germanium
Authors demonstrate the synthesis and characterization of direct bandgap quantum wells in the hexagonal Si1−xGex system. Photoluminescence experiments show light emission up to room temperature, and the emission wavelength can be tuned by thickness of the wells and the Si composition.
- Wouter H. J. Peeters
- , Victor T. van Lange
- & Erik P. A. M. Bakkers
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Article
| Open AccessBulk-suppressed and surface-sensitive Raman scattering by transferable plasmonic membranes with irregular slot-shaped nanopores
Characterizing surfaces by Raman spectroscopy is limited by the competition of surface and bulk Raman responses. Here the authors use nanoporous plasmonic membranes to enhance surface Raman signals while suppressing bulk contributions.
- Roman M. Wyss
- , Günter Kewes
- & Sebastian Heeg
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Article
| Open AccessStrain to shine: stretching-induced three-dimensional symmetries in nanoparticle-assembled photonic crystals
Understanding the deformation of nanoparticle lattices in elastic materials is crucial for photonics. Here, authors reveal 3D lattice transformations under strain with models and experiments, demonstrating tuneable optical properties and significant structural changes.
- Tong An
- , Xinyu Jiang
- & Qibin Zhao
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Article
| Open AccessUltrabright and stable top-emitting quantum-dot light-emitting diodes with negligible angular color shift
By improving the method of determining the penetration depth, lowering film refractive indices, and narrowing emission linewidth, Li et al. report single mode top-emitting green QLEDs with EQE of 29.2%, luminance of 1.6 million nits, T95 of 15,600 h at 1000 nits, and negligible angular colour shift.
- Mengqi Li
- , Rui Li
- & Song Chen
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Article
| Open AccessScanless two-photon voltage imaging
Detection of membrane potential changes using voltage indicators typically requires fast imaging rates and highly sensitive imaging methods. Here, the authors introduce scanless two-photon imaging, an approach which enables high signal to noise ratio voltage recordings at kilohertz rates, from multiple neurons simultaneously, both in vitro and in vivo.
- Ruth R. Sims
- , Imane Bendifallah
- & Valentina Emiliani
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Article
| Open AccessNanoscale optical nonreciprocity with nonlinear metasurfaces
Here the authors develop a subwavelength nonreciprocal optical component harnessing the effect is thermal phase transition of VO2 boosted by the Mie resonant response of the dielectric meta-surface.
- Aditya Tripathi
- , Chibuzor Fabian Ugwu
- & Sergey S. Kruk
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Article
| Open AccessMicro-optical elements from optical-quality ZIF-62 hybrid glasses by hot imprinting
Hybrid MOF-glasses can be shaped and processed in analogy to conventional glasses. Here, microstructures are formed by thermal imprinting, whilst preserved porosity of the material enables its further use in responsive optics.
- Oksana Smirnova
- , Roman Sajzew
- & Lothar Wondraczek
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Article
| Open AccessAxial de-scanning using remote focusing in the detection arm of light-sheet microscopy
The authors propose a method for de-scanning the axial focus movement in the detection arm of a fluorescence microscope, enabling aberration-free, multi-color, volumetric imaging. They acquire dual-colour image stacks with an axial range of 70 μm and camera-limited acquisition speed.
- Hassan Dibaji
- , Ali Kazemi Nasaban Shotorban
- & Tonmoy Chakraborty
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Article
| Open AccessDispersive Fourier transform based dual-comb ranging
Here the authors develop a dispersive Fourier transform (DFT) based LIDAR method utilizing phase-locked Vernier dual soliton laser combs and demonstrate improved precision in the measurements.
- Bing Chang
- , Teng Tan
- & Baicheng Yao
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Article
| Open AccessAll-optical phase conjugation using diffractive wavefront processing
The authors present a diffractive optical processor that approximates optical phase conjugation operation without any digital computing. This compact and all-optical wavefront processor can be used for various applications, including turbidity suppression and aberration correction.
- Che-Yung Shen
- , Jingxi Li
- & Aydogan Ozcan
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Article
| Open AccessQuantum coherence and interference of a single moiré exciton in nano-fabricated twisted monolayer semiconductor heterobilayers
Here, the authors develop a microfabrication method to realize the optical observation of quantum coherence and interference of a single moiré exciton in twisted semiconducting heterobilayers of transition metal dichalcogenides, persisting beyond 10 ps.
- Haonan Wang
- , Heejun Kim
- & Kazunari Matsuda
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Article
| Open AccessIntrinsically stretchable organic photovoltaics by redistributing strain to PEDOT:PSS with enhanced stretchability and interfacial adhesion
The realization of intrinsically stretchable organic photovoltaics with excellent mechanical robustness remains challenging. Here, the authors redistribute the strain in the active layer to PEDOT:PSS electrodes with simultaneously enhanced stretchability and interfacial adhesion in the device.
- Jiachen Wang
- , Yuto Ochiai
- & Takao Someya
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Article
| Open AccessNondiffracting supertoroidal pulses and optical “Kármán vortex streets”
Topological waves and their exotic properties are attracting intense research interest. Here, the authors report on the discovery of supertoroidal electromagnetic pulses with robust skyrmionic topology that persists upon propagation over arbitrarily long distances.
- Yijie Shen
- , Nikitas Papasimakis
- & Nikolay I. Zheludev
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Article
| Open AccessDepth-enhanced high-throughput microscopy by compact PSF engineering
Implementing point spread function (PSF) engineering in high-throughput microscopy has proved challenging. Here, the authors propose a compact PSF engineering approach, which allows for enhanced depth of field and for the recovery of 3D information using single snapshots.
- Nadav Opatovski
- , Elias Nehme
- & Yoav Shechtman
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Article
| Open AccessDiscovery of atomic clock-like spin defects in simple oxides from first principles
Recently, long spin coherence times have been predicted for spin defects in simple oxides. Here, by using high-throughput first-principles calculations, the authors identify promising spin defects in CaO, with electronic properties similar to those of NV centers but with longer coherence times.
- Joel Davidsson
- , Mykyta Onizhuk
- & Giulia Galli
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Article
| Open AccessHighly confined epsilon-near-zero and surface phonon polaritons in SrTiO3 membranes
Transition metal perovskite oxide membranes are promising platforms for infrared polaritonics. Here, the authors experimentally demonstrate highly confined epsilon-near-zero modes and propagating surface phonon polaritons in high-quality SrTiO3 membranes with deep subwavelength thickness.
- Ruijuan Xu
- , Iris Crassee
- & Yin Liu
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Article
| Open AccessStretchable OLEDs based on a hidden active area for high fill factor and resolution compensation
The reduction in geometrical fill factor in stretchable organic light-emitting diodes (OLEDs) limits their potential for applications. Here, authors report a 3D architecture adopting a hidden active area as both emitting area and interconnector, realizing OLEDs with high post-stretch fill factor.
- Donggyun Lee
- , Su-Bon Kim
- & Seunghyup Yoo
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Article
| Open AccessHigh-resolution, large field-of-view label-free imaging via aberration-corrected, closed-form complex field reconstruction
The authors present APIC, a closed-form reconstruction method for microscopy that avoids iterative algorithms, enabling correct imaging reconstruction with no additional hardware. APIC demonstrates analytical complex field reconstructions from darkfield measurements and NA-matching alone.
- Ruizhi Cao
- , Cheng Shen
- & Changhuei Yang
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Article
| Open AccessObservation of nonlinear response and Onsager regression in a photon Bose-Einstein condensate
Perturbing a physical system, for example, picking a guitar string to make it vibrate, tells a lot about its intrinsic properties. Here the authors show that such concepts hold even for quantum gases of light, which respond to a perturbation with the same dynamics as they fluctuate on their own.
- Alexander Sazhin
- , Vladimir N. Gladilin
- & Julian Schmitt
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Article
| Open AccessIn-situ observation of silk nanofibril assembly via graphene plasmonic infrared sensor
Here, the authors develop a graphene plasmonic infrared sensor to probe the secondary structure of nanoscale assembly intermediates and the morphological evolution of silk nanofibrils, the fundamental building blocks of silk fibres.
- Chenchen Wu
- , Yu Duan
- & Qing Dai
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Article
| Open AccessBroadband near-infrared emission in silicon waveguides
On-chip optical sensing and metrology systems are rapidly progressing, but CMOS-compatible silicon light sources remain a challenge. This work demonstrates a broadband, foundry integrated silicon waveguide emitter and the theory that describes it.
- Marcel W. Pruessner
- , Nathan F. Tyndall
- & Todd H. Stievater
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Article
| Open AccessPhotoinduced dynamics during electronic transfer from narrow to wide bandgap layers in one-dimensional heterostructured materials
One-dimensional van der Waals heterostructures can realize atomically thin transistor junctions. Here, the authors study electron transfer in such layered structures using ultrafast diffraction and spectroscopy as well as theoretical simulations.
- Yuri Saida
- , Thomas Gauthier
- & Masaki Hada
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Article
| Open AccessHigh-speed optical imaging with sCMOS pixel reassignment
The authors introduce a highspeed acquisition technique, sHAPR, for rapid exploration of biodynamics using fluorescence microscopy. The method leverages sCMOS cameras and custom fibre optics to convert microscopy images into 1D recordings, enabling acquisition at the maximum camera readout rate.
- Biagio Mandracchia
- , Corey Zheng
- & Shu Jia
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Article
| Open AccessObservation of the photonic Hall effect and photonic magnetoresistance in random lasers
This work reveals the presence of the photonic Hall effect and photonic magnetoresistance in a field-dependent random laser. This observation visualizes the influence of magnetic field on random lasers scattering at the microscopic level.
- Wenyu Du
- , Lei Hu
- & Zhijia Hu
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Article
| Open AccessOrganic and inorganic sublattice coupling in two-dimensional lead halide perovskites
By resonant pumping the organic cation in 2D perovskite, Fu et al. report the electronic and mechanical couplings between the organic and inorganic sublattices, evidenced by the reduced bandgap and modified lattice degree of freedom within the inorganic sublattice, and slow heat transfer process.
- Jianhui Fu
- , Tieyuan Bian
- & Tze Chien Sum
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Article
| Open AccessDirectional thermal emission and display using pixelated non-imaging micro-optics
The authors demonstrate ultrabroadband, polarisation-independent directional control of thermal radiation using a pixelated micro-emitter, and produce large emissivity contrast at different directions, with potential applications to radiative cooling, infrared spectroscopy and thermophotovoltaics.
- Ziwei Fan
- , Taeseung Hwang
- & Zi Jing Wong
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Article
| Open AccessMicrowave-transparent metallic metamaterials for autonomous driving safety
Lee et al. developed ultrathin metallic (metal filling ratios of > 70 %) metamaterials that exhibit perfect transmission at a specific radar frequency. These characteristics enable microwave transparent, low-sheet-resistance radar heaters for safe autonomous driving in extreme weather.
- Eun-Joo Lee
- , Jun-Young Kim
- & Sun-Kyung Kim
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Article
| Open AccessNarrowband room temperature phosphorescence of closed-loop molecules through the multiple resonance effect
Luminescent materials with narrowband emissions are vital for optoelectronic applications. Here, the authors achieve room temperature phosphorescence with a FWHM of 30 nm through the multiple resonance effect and showcase its practical application in X-ray imaging.
- Xiaokang Yao
- , Yuxin Li
- & Zhongfu An
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Article
| Open AccessQuantum barriers engineering toward radiative and stable perovskite photovoltaic devices
Efficient radiation is essential to reach thermodynamic limit of photovoltaic efficiency. Here, authors design thick quantum barriers to suppress interfacial quenching and boost photon recycling in perovskite cells, achieving high radiation and photovoltaic efficiencies and long device stability.
- Kyung Mun Yeom
- , Changsoon Cho
- & Jun Hong Noh
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Article
| Open AccessIntegrated photonic encoder for low power and high-speed image processing
The researchers showcase a silicon-photonics-based analog approach for large-scale image processing that can be deployed for high-speed image compression and de-noising using an auto-encoder framework with minimal power consumption.
- Xiao Wang
- , Brandon Redding
- & Raktim Sarma